Dioxin removal systems for waste gases
AGC Engineering Co. of Japan has developed a dioxin removal system based on activated carbon. The process basically involves injecting 0.1-0.2 g/Nm3 activated carbon relative to the amount of waste gas. AGC Engineering says that the system guarantees a toxicity equivalent of 0.5 ng/Nm3 or less at inlet of the bag filter, and less than 0.1 ng/Nm3 after bag filter process with catalyst device. The system can be designed to use activated carbon mixed with slaked lime, if needed. The catalyst employed is plate-type, with opening widths of 4 mm or 6 mm.


Contact: AGC Engineering Co. Ltd., WBG Marive West, 19th Floor, 6 Nakase 2-chome, Mihama-ku, Chiba-shi, Chiba 261-7119, Japan.


Source: www.agec.co.jp 
Catalytic removal of nitro-PAHs
Siemens Aktiengesellschaft, based in Germany, has been assigned a United States patent on a process for the catalytic removal of polycyclic aromatic nitro, nitroso and/or amino compounds (nitrated polycyclic aromatic hydrocarbons – nitro-PAHs) from the exhaust gas of a combustion system, in particular a diesel engine. The exhaust gas is brought into contact with a catalytic converter at a temperature of from 150º to 600ºC. The nitro-PAHs are oxidized at the catalytic converter through the use of oxygen to form nitrogen oxides (NOx), carbon dioxide (CO2) and water.


The catalytic material contains, by weight, 80 to 95 per cent titanium dioxide, 2 to 10 per cent tungsten trioxide or molybdenum trioxide, and 0.05 to 5 per cent vanadium pentoxide. To oxidize the nitro-PAHs, a certain oxygen content is required in the exhaust gas. The exhaust gas of a diesel engine is inherently high in residual oxygen content.


In one of the configurations, a reducing agent containing nitrogen is added to the exhaust gas before it is brought into contact with the catalytic converter in the presence of oxygen to reduce NOx contained in the exhaust gas. In this way, first the formation of the nitro-PAHs from PAHs and NOx in the exhaust gas is prevented.


Second, the catalytic converter is used as a deNOx catalytic converter for the removal of NOx using the SCR process. Also, nitro-PAHs are converted at the catalytic converter, together with oxygen and the nitrogen-containing reducing agent, to form non-hazardous compounds. This is a reaction pathway in addition to the oxidation of the nitro-PAHs with oxygen to form CO2 and water.


Source: www.freepatentsonline.com
PAH removal from spiked municipal sewage sludge
Researchers from the Institute of Scientific Research, University of Québec, Canada, studied different processes for removing polycyclic aromatic hydrocarbons (PAHs) from municipal sewage sludge and wastewater. PAHs are strongly adsorbed on to particulate matters of soils, sludge or sediments owing to their strong hydrophobicity, which makes them less “bio-available”, thus limiting their bioremediation.


Using sludge doped with 11 PAHs at 5.5 mg of each PAH per kg of dry matter, the scientists tested different treatment processes to evaluate the PAH removal performance of each. Two biological processes – mesophilic aerobic digestion (MAD) and simultaneous sewage sludge digestion and metal leaching (METIX-BS) – were tested to evaluate PAH biodegradation in sewage sludge. In parallel, two quite similar chemical Fenton processes – chemical metal leaching (METIX-AC) and chemical stabilization (STABIOX) – and one electrochemical stabilization process (ELECSTAB) were tested to measure PAH removal by these oxidative processes. Moreover, PAH solubilization from sludge by the addition of a non-ionic surfactant Tween 80 (Tw80) was also tested.


The best PAH removal rates were obtained by MAD and METIX-BS with more than 95 per cent 3-ring PAH removal after 21 days of treatment.


Addition of Tw80 during MAD treatment increased removal rate of 4-ring PAHs. More than 45 per cent of 3-ring PAHs were removed from sludge by METIX-AC, while about 62 per cent of 3-ring PAHs were removed by ELECSTAB process. However, STABIOX process showed only <35 per cent removal of 3-ring PAHs. None of the processes were efficient for the elimination of high molecular weight PAHs (5-ring or above) from sludge.


Source: www.ncbi.nlm.nih.gov
Biodegradation of PAHs in petroleum-contaminated soil
Scientists at the National Research Centre for Environmental and Hazardous Waste Management, Thailand, investigated bioremediation of polycyclic aromatic hydrocarbons (PAHs) in petroleum-contaminated soil using tamarind leaf inoculums. Leaves of tamarind and other leguminous trees have been reported to contain several PAH-degrading micro-organisms.


To minimize the amount of leaves added, tamarind leaf inoculums were prepared by incubating the leaves with a sub-sample of contaminated soil for 49 days. Then the efficiency of the inoculums was tested with two soil samples collected from a navy dockyard and railway station. These soil samples had different levels of petroleum contamination. Bioaugmentation treatment was carried out by mixing contaminated soil with the inoculums at the ratio of 9:1. For navy dockyard soil, the concentration of phenanthrene in the inoculated soil was reduced gradually to undetectable level within 56 days; 70-80 per cent of fluoranthene and pyrene remained at the end of the treatment. For railway station soil, which had lower petroleum contamination, PAH degradation occurred faster: the phenanthrene concentration was below detection limit after 28 days.


The treatment also succeeded in reducing the quantities of several hydrocarbons. At the same time, numerous phenanthrene-degrading bacteria, which were used as representatives of PAH degraders, could be observed in both inoculated soils. Higher numbers of bacteria, however, were found in railway station soil, which corresponded with the lower amount of PAHs and higher amount of soil nutrients. The results showed that inoculums prepared from tamarind leaves could be used to degrade PAHs as well as clean-up petroleum contaminated soil.


Source: www.psu.ac.th 
Promising discovery for PCB clean-up without dredging
Dr. Donna Bedard at the Rensselaer Polytechnic Institute and scientists from Georgia Institute of Technology, the United States, have discovered a bacterium that could remove polychlorinated biphenyls (PCBs) from the environment without dredging. The discovery is a first step towards a bioremediation strategy to naturally detoxify the chemicals without risky removal of the sediments in which they persist. Dr. Bedard, describing the potential breakthrough, said the research will help scientists understand the process by which PCBs have been known to break down naturally in water.


In microcosm studies in her lab, Dr. Bedard found that Aroclor 1260 was being degraded by native sediment microbes. She developed sediment-free enrichment cultures, characterized them in collaboration with Dr. Frank Loeffler and Dr. Kirsti Ritalahti of GeogiaTech. After a series of experiments, the team was able to determine that bacteria in the Dehalococcoides (Dhc) group were responsible for the dechlorination of Aroclor 1260. These microbes replace the chlorine atoms in Aroclor 1260 with hydrogen, which fuels their growth and initiates the PCB degradation process.


Source: www.gtresearchnews.gatech.edu 
Sorbent to prevent dioxin synthesis
DIOX-BLOK® from Beco Engineering Company, the United States, is a patented sorbent that prevents new dioxin synthesis in combustion processes. Although modern incineration processes completely destroy dioxins, they form anew as the flue gas cools below 400ºC. On cool-down, trace organics adsorb on the fly-ash and are converted to dioxins by reaction with the metal chlorides on the surface of the ash.
DIOX-BLOK achieves two things:
 
  • It “starves” the fly-ash of dioxin reactants by removing organics before they can be adsorbed by the ash; and
     
  • Dioxin-contaminated ash is not created: unlike powdered activated carbon (PAC), DIOX-BLOK is chemically inert and adsorbed organics are not converted to dioxins.
     

DIOX-BLOK is used at rates of from 450-900 g/t of waste burned. The delivered cost of is generally less than, or equal to, the cost of PAC.


Besides, as prevents dioxins from forming, its environmental cost is far less than PAC. Its use with medical / hazardous / municipal waste inci-nerators in dry / wet scrubber units has reportedly shown good results, reducing dioxin emissions to 0.001-0.006 ng/dscm, TEQ.


Contact: Beco Engineering Company, P.O. Box 443, 800 3rd Street, Oakmont, PA 15139, United States of America. Fax: +1 (412) 828 6144


E-mail: becoengco@aol.com


Source: www.becoengineering.com